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Micromechanical modelling of alumina trihydrate filled poly (methyl methacrylate) composites

Published Online:pp 31-47https://doi.org/10.1504/IJMSI.2013.055106

The microstructure of a binary composite consisting of stiff particles embedded in a matrix was modelled using finite element analysis. A regular square mesh was generated and an image of the microstructure was used to assign the appropriate material parameters to each integration point depending on its location relative to the original image. The same image was also used to find the particle size distribution of the filler which was used to recreate a simulated microstructure with the same volume fraction. The simulated microstructure represented the filler particles as circles with diameters ranging from 1 μm to 95 μm. The size and position of each filler particle was used to generate a model by explicitly meshing each particle boundary. The simulated microstructure reproduced the same strain values under tension as the original microstructural image, the implication being that it is possible to model a microstructure when a clear image is not available provided statistical size distribution data is available. The predicted composite modulus was compared to experimental values obtained from tensile tests available in the literature and to analytic predictions. The strain fields were compared to digital image correlation analysis of images obtained from tensile tests performed using in-situ SEM.

Keywords

binary composites, ATH, PMMA, micromechanical modelling, DIC

References

  • 1. Benveniste, Y. (1987). ‘A new approach to the application of Mori-Tanaka’s theory in composite materials’. Mechanics of Materials. 6, 2, 147-157 Google Scholar
  • 2. Buryachenko, V.A. , Pagano, N.J. , Kim, R.Y. , Spowart, E. (2003). ‘Quantitative description and numerical simulation of random microstructures of composites and their effective elastic moduli’. International Journal of Solids and Structures. 40, 1, 47-52 Google Scholar
  • 3. Chen, Q. , Chasiotis, I. , Chen, C. , Roy, A. (2008). ‘Nanoscale and effective mechanical behavior and fracture of silica nanocomposites’. Composites Science and Technology. 68, 15–16, 3137-3144 Google Scholar
  • 4. Christensen, R.M. (1990). ‘A critical evaluation for a class of micro-mechanics models’. Journal of the Mechanics and Physics of Solids. 38, 3, 379-404 Google Scholar
  • 5. Eshelby, J.D. (1957). ‘The determination of the elastic field of an ellipsoidal inclusion and related problems’. Proceedings of the Royal Society of London. A241, 1226, 376-396 Google Scholar
  • 6. Ferreira, J.M. , Costa, J.D. , Capela, C. (1997). ‘Fracture assessment of PMMA/Si kitchen sinks made from acrylic casting dispersion’. Theoretical and Applied Fracture Mechanics. 26, 2, 105-116 Google Scholar
  • 7. Hashin, Z. , Shtrikman, S. (1963). ‘A variational approach to the theory of the elastic behaviour of multiphase materials’. Journal of the Mechanics and Physics of Solids. 11, 2, 127-140 Google Scholar
  • 8. Liang, J.Z. , Li, R.K.Y. (1998). ‘Prediction of tensile yield strength of rigid inorganic particulate filled thermoplastic composites’. Journal of Materials Processing Technology. 83, 1, 127-130 Google Scholar
  • 9. Lielens, G. , Keunings, R. (1999). ‘Prediction of flow-induced physical properties of short fiber composites’. Proceedings of the 7th European Conference on Composite Materials: Realising Their Commercial Potential. 14–16 May, London, UK, 51-56 Google Scholar
  • 10. Milton, G.W. (1981). ‘Bounds on the electromagnetic, elastic and other properties of two-component composites’. Physical Review Letters. 46, 8, 542-545 Google Scholar
  • 11. Nie, S. , Basaran, C. (2005). ‘A micromechanical model for effective elastic properties of particulate composites with imperfect interfacial bonds’. International Journal of Solids and Structures. 42, 14, 4179-4191 Google Scholar
  • 12. Regino, M. , Busso, E.P. , O’Dowd, N.P. , Allen, D. ‘A multiscale constitutive approach to model the mechanical behaviour of inhomogeneous single crystal superalloys’. Proceedings of the 7th Liege Conference on Materials for Advanced Power Engineering. 2002, 09, Liege, Belgium, 283-291 Google Scholar
  • 13. Rothon, R.N. (1995). ‘Particulate-filled polymer composites’. Polymer Science and Technology Series. Harlow, Essex:Longman Scientific & Technical Google Scholar
  • 14. Stapountzi, O.A. , Charalambides, M.N. , Williams, J.G. (2009). ‘Micromechanical models for stiffness prediction of alumina trihydrate (ATH) reinforced poly (methyl methacrylate) (PMMA): effect of filler volume fraction and temperature’. Composites Science and Technology. 69, 11–12, 2015-2023 Google Scholar
  • 15. Stapountzi, O.A. , Charalambides, M.N. , Williams, J.G. (2010). ‘The fracture toughness of a highly filled polymer composite’. Recent Advances in Mechanics. Netherlands:Springer Google Scholar
  • 16. Tan, H. , Liu, C. , Geubelle, P.H. (2005). ‘The cohesive law for the particle/matrix interfaces in high explosives’. Journal of the Mechanics and Physics of Solids. 53, 8, 1892-1917 Google Scholar
  • 17. Tandon, G.P. , Weng, G.J. (1984). ‘The effect of aspect ratio of inclusions on the elastic properties of unidirectionally aligned composites’. Polymer Composites. 5, 4, 327-333 Google Scholar
  • 18. Tucker, C.L., III , Liang, E. (1999). ‘Stiffness predictions for unidirectional short-fiber composites: review and evaluation’. Composites Science and Technology. 59, 5, 655-671 Google Scholar
  • 19. Walpole, L.J. (1966). ‘On bounds for the overall elastic moduli of inhomogeneous systems I’. Journal of the Mechanics and Physics of Solids. 14, 3, 151-162 Google Scholar
  • 20. Wolodko, J.D. , Xia, Z. , Ellyin, F. (2000). ‘Analysis of Al/Al2O3 metal matrix composites under biaxial cyclic loading using a digital image based finite element method’. Materials Science and Technology. 16, 7–8, 837-842 Google Scholar
  • 21. Zhang, B. , Yang, Z. , Sun, X. , Tang, Z. (2010). ‘A virtual experimental approach to estimate composite mechanical properties: modeling with an explicit finite element method’. Computational Materials Science. 49, 3, 645-651 Google Scholar

Addirional References